Did you read the article in the link PeterOz posted?
You can't play music CDs or DVD videos with a Chromebook DVD drive....ChromeOS does not support optical disks to let you play music or movies. The primary reason for this is that Chrome OS doesn't come with codecs. Codecs are necessary to compress and decompress large files like DVD videos.
Since you downloaded VLC, I assume you wished to play an audio or video DVD which won't work.
One article implies you can use an external optical drive to play music and movies while the other implies it can only be used for data.
The article that says you can tells you to put the DVD into the drive before you attach it to the Chromebook. Have you tried that?
What are the manufacturers and exact model numbers of the Chrome book and DVD drive?
What release of Chrome are you running?
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